Influence of Wooden Sawdust Treatments on Cu(II) and Zn(II) Removal from Water.
Identifieur interne : 000318 ( Main/Exploration ); précédent : 000317; suivant : 000319Influence of Wooden Sawdust Treatments on Cu(II) and Zn(II) Removal from Water.
Auteurs : Zdenka Kovacova [Slovaquie] ; Stefan Demcak [Slovaquie] ; Magdalena Balintova [Slovaquie] ; Cocencepcion Pla [Espagne] ; Inga Zinicovscaia [Russie, Roumanie]Source :
- Materials (Basel, Switzerland) [ 1996-1944 ] ; 2020.
Abstract
Organic waste materials and semi-products containing cellulose are used as low-cost adsorbents that are able to compete with conventional sorbents. In addition, their capacity to bind heavy metal ions can be intensified by chemical treatments using mineral and organic acids, bases, oxidizing agents, and organic compounds. In this paper, we studied the biosorption capacity of natural and modified wooden sawdust of poplar, cherry, spruce, and hornbeam in order to remove heavy metals from acidic model solutions. The Fourier transform infrared spectroscopy (FTIR) spectra showed changes of the functional groups due to the alkaline modification of sawdust, which manifested in the considerably increased intensity of the hydroxyl peaks. The adsorption isotherm models clearly indicated that the adsorptive behavior of metal ions in treated sawdust satisfied not only the Langmuir model, but also the Freundlich model. The adsorption data obtained for studied sorbents were better fitted by the Langmuir isotherm model for both metals, except for spruce sawdust. Surface complexation and ion exchange are the major mechanisms involved in metal ion removal. We investigated the efficiency of the alkaline modified sawdust for metal removal under various initial concentrations of Cu(II) and Zn(II) from model solutions. The highest adsorption efficiency values (copper 94.3% at pH 6.8 and zinc 98.2% at pH 7.3) were obtained for poplar modified by KOH. For all types of sawdust, we found that the sorption efficiency of modified sorbents was higher in comparison to untreated sawdust. The value of the pH initially increased more in the case of modified sawdust (8.2 for zinc removal with spruce NaOH) and then slowly decreased (7.0 for Zn(II) with spruce NaOH).
DOI: 10.3390/ma13163575
PubMed: 32823585
PubMed Central: PMC7476008
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Kosice</wicri:noRegion></affiliation></author><author><name sortKey="Demcak, Stefan" sort="Demcak, Stefan" uniqKey="Demcak S" first="Stefan" last="Demcak">Stefan Demcak</name><affiliation wicri:level="1"><nlm:affiliation>Faculty of Civil Engineering, Institute of Environmental Engineering, Technical University of Kosice, Vysokoskolska 4, 042 00 Kosice, Slovakia.</nlm:affiliation><country xml:lang="fr">Slovaquie</country><wicri:regionArea>Faculty of Civil Engineering, Institute of Environmental Engineering, Technical University of Kosice, Vysokoskolska 4, 042 00 Kosice</wicri:regionArea><wicri:noRegion>042 00 Kosice</wicri:noRegion></affiliation></author><author><name sortKey="Balintova, Magdalena" sort="Balintova, Magdalena" uniqKey="Balintova M" first="Magdalena" last="Balintova">Magdalena Balintova</name><affiliation wicri:level="1"><nlm:affiliation>Faculty of Civil Engineering, Institute of Environmental Engineering, Technical University of Kosice, Vysokoskolska 4, 042 00 Kosice, Slovakia.</nlm:affiliation><country xml:lang="fr">Slovaquie</country><wicri:regionArea>Faculty of Civil Engineering, Institute of Environmental Engineering, Technical University of Kosice, Vysokoskolska 4, 042 00 Kosice</wicri:regionArea><wicri:noRegion>042 00 Kosice</wicri:noRegion></affiliation></author><author><name sortKey="Pla, Cocencepcion" sort="Pla, Cocencepcion" uniqKey="Pla C" first="Cocencepcion" last="Pla">Cocencepcion Pla</name><affiliation wicri:level="2"><nlm:affiliation>Department of Civil Engineering, University of Alicante, Carretera de s/n, 03690 Alicante, Spain.</nlm:affiliation><country xml:lang="fr">Espagne</country><wicri:regionArea>Department of Civil Engineering, University of Alicante, Carretera de s/n, 03690 Alicante</wicri:regionArea><placeName><region nuts="2" type="communauté">Communauté valencienne</region></placeName></affiliation></author><author><name sortKey="Zinicovscaia, Inga" sort="Zinicovscaia, Inga" uniqKey="Zinicovscaia I" first="Inga" last="Zinicovscaia">Inga Zinicovscaia</name><affiliation wicri:level="1"><nlm:affiliation>Joint Institute for Nuclear Research, Joliot-Curie Str. 6, 1419890 Dubna, Russia.</nlm:affiliation><country xml:lang="fr">Russie</country><wicri:regionArea>Joint Institute for Nuclear Research, Joliot-Curie Str. 6, 1419890 Dubna</wicri:regionArea><wicri:noRegion>1419890 Dubna</wicri:noRegion></affiliation><affiliation wicri:level="1"><nlm:affiliation>Horia Hulubei National Institute for R&D in Physics and Nuclear Engineering, 30 Reactorului Str., MG-6, Bucharest, 077125 Magurele, Romania.</nlm:affiliation><country xml:lang="fr">Roumanie</country><wicri:regionArea>Horia Hulubei National Institute for R&D in Physics and Nuclear Engineering, 30 Reactorului Str., MG-6, Bucharest, 077125 Magurele</wicri:regionArea><wicri:noRegion>077125 Magurele</wicri:noRegion></affiliation></author></analytic><series><title level="j">Materials (Basel, Switzerland)</title><idno type="ISSN">1996-1944</idno><imprint><date when="2020" type="published">2020</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">Organic waste materials and semi-products containing cellulose are used as low-cost adsorbents that are able to compete with conventional sorbents. In addition, their capacity to bind heavy metal ions can be intensified by chemical treatments using mineral and organic acids, bases, oxidizing agents, and organic compounds. In this paper, we studied the biosorption capacity of natural and modified wooden sawdust of poplar, cherry, spruce, and hornbeam in order to remove heavy metals from acidic model solutions. The Fourier transform infrared spectroscopy (FTIR) spectra showed changes of the functional groups due to the alkaline modification of sawdust, which manifested in the considerably increased intensity of the hydroxyl peaks. The adsorption isotherm models clearly indicated that the adsorptive behavior of metal ions in treated sawdust satisfied not only the Langmuir model, but also the Freundlich model. The adsorption data obtained for studied sorbents were better fitted by the Langmuir isotherm model for both metals, except for spruce sawdust. Surface complexation and ion exchange are the major mechanisms involved in metal ion removal. We investigated the efficiency of the alkaline modified sawdust for metal removal under various initial concentrations of Cu(II) and Zn(II) from model solutions. The highest adsorption efficiency values (copper 94.3% at pH 6.8 and zinc 98.2% at pH 7.3) were obtained for poplar modified by KOH. For all types of sawdust, we found that the sorption efficiency of modified sorbents was higher in comparison to untreated sawdust. The value of the pH initially increased more in the case of modified sawdust (8.2 for zinc removal with spruce NaOH) and then slowly decreased (7.0 for Zn(II) with spruce NaOH).</div></front></TEI><pubmed><MedlineCitation Status="PubMed-not-MEDLINE" Owner="NLM"><PMID Version="1">32823585</PMID><DateRevised><Year>2020</Year><Month>09</Month><Day>28</Day></DateRevised><Article PubModel="Electronic"><Journal><ISSN IssnType="Print">1996-1944</ISSN><JournalIssue CitedMedium="Print"><Volume>13</Volume><Issue>16</Issue><PubDate><Year>2020</Year><Month>Aug</Month><Day>13</Day></PubDate></JournalIssue><Title>Materials (Basel, Switzerland)</Title><ISOAbbreviation>Materials (Basel)</ISOAbbreviation></Journal><ArticleTitle>Influence of Wooden Sawdust Treatments on Cu(II) and Zn(II) Removal from Water.</ArticleTitle><ELocationID EIdType="pii" ValidYN="Y">E3575</ELocationID><ELocationID EIdType="doi" ValidYN="Y">10.3390/ma13163575</ELocationID><Abstract><AbstractText>Organic waste materials and semi-products containing cellulose are used as low-cost adsorbents that are able to compete with conventional sorbents. In addition, their capacity to bind heavy metal ions can be intensified by chemical treatments using mineral and organic acids, bases, oxidizing agents, and organic compounds. In this paper, we studied the biosorption capacity of natural and modified wooden sawdust of poplar, cherry, spruce, and hornbeam in order to remove heavy metals from acidic model solutions. The Fourier transform infrared spectroscopy (FTIR) spectra showed changes of the functional groups due to the alkaline modification of sawdust, which manifested in the considerably increased intensity of the hydroxyl peaks. The adsorption isotherm models clearly indicated that the adsorptive behavior of metal ions in treated sawdust satisfied not only the Langmuir model, but also the Freundlich model. The adsorption data obtained for studied sorbents were better fitted by the Langmuir isotherm model for both metals, except for spruce sawdust. Surface complexation and ion exchange are the major mechanisms involved in metal ion removal. We investigated the efficiency of the alkaline modified sawdust for metal removal under various initial concentrations of Cu(II) and Zn(II) from model solutions. The highest adsorption efficiency values (copper 94.3% at pH 6.8 and zinc 98.2% at pH 7.3) were obtained for poplar modified by KOH. For all types of sawdust, we found that the sorption efficiency of modified sorbents was higher in comparison to untreated sawdust. The value of the pH initially increased more in the case of modified sawdust (8.2 for zinc removal with spruce NaOH) and then slowly decreased (7.0 for Zn(II) with spruce NaOH).</AbstractText></Abstract><AuthorList CompleteYN="Y"><Author ValidYN="Y"><LastName>Kovacova</LastName><ForeName>Zdenka</ForeName><Initials>Z</Initials><AffiliationInfo><Affiliation>Faculty of Civil Engineering, Institute of Environmental Engineering, Technical University of Kosice, Vysokoskolska 4, 042 00 Kosice, Slovakia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Demcak</LastName><ForeName>Stefan</ForeName><Initials>S</Initials><Identifier Source="ORCID">0000-0001-6660-6142</Identifier><AffiliationInfo><Affiliation>Faculty of Civil Engineering, Institute of Environmental Engineering, Technical University of Kosice, Vysokoskolska 4, 042 00 Kosice, Slovakia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Balintova</LastName><ForeName>Magdalena</ForeName><Initials>M</Initials><Identifier Source="ORCID">0000-0002-5644-2866</Identifier><AffiliationInfo><Affiliation>Faculty of Civil Engineering, Institute of Environmental Engineering, Technical University of Kosice, Vysokoskolska 4, 042 00 Kosice, Slovakia.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Pla</LastName><ForeName>Cocencepcion</ForeName><Initials>C</Initials><Identifier Source="ORCID">0000-0002-4269-2426</Identifier><AffiliationInfo><Affiliation>Department of Civil Engineering, University of Alicante, Carretera de s/n, 03690 Alicante, Spain.</Affiliation></AffiliationInfo></Author><Author ValidYN="Y"><LastName>Zinicovscaia</LastName><ForeName>Inga</ForeName><Initials>I</Initials><Identifier Source="ORCID">0000-0003-0820-887X</Identifier><AffiliationInfo><Affiliation>Joint Institute for Nuclear Research, Joliot-Curie Str. 6, 1419890 Dubna, Russia.</Affiliation></AffiliationInfo><AffiliationInfo><Affiliation>Horia Hulubei National Institute for R&D in Physics and Nuclear Engineering, 30 Reactorului Str., MG-6, Bucharest, 077125 Magurele, Romania.</Affiliation></AffiliationInfo></Author></AuthorList><Language>eng</Language><GrantList CompleteYN="Y"><Grant><GrantID>1/0419/19</GrantID><Agency>VEGA - Scientific Grant Agency of the Ministry of Education</Agency><Country></Country></Grant></GrantList><PublicationTypeList><PublicationType UI="D016428">Journal Article</PublicationType></PublicationTypeList><ArticleDate DateType="Electronic"><Year>2020</Year><Month>08</Month><Day>13</Day></ArticleDate></Article><MedlineJournalInfo><Country>Switzerland</Country><MedlineTA>Materials (Basel)</MedlineTA><NlmUniqueID>101555929</NlmUniqueID><ISSNLinking>1996-1944</ISSNLinking></MedlineJournalInfo><KeywordList Owner="NOTNLM"><Keyword MajorTopicYN="N">Freundlich isotherm</Keyword><Keyword MajorTopicYN="N">Langmuir isotherm</Keyword><Keyword MajorTopicYN="N">alkaline modification</Keyword><Keyword MajorTopicYN="N">heavy metals</Keyword><Keyword MajorTopicYN="N">sorption</Keyword><Keyword MajorTopicYN="N">wooden sawdust</Keyword></KeywordList></MedlineCitation><PubmedData><History><PubMedPubDate PubStatus="received"><Year>2020</Year><Month>07</Month><Day>01</Day></PubMedPubDate><PubMedPubDate PubStatus="revised"><Year>2020</Year><Month>08</Month><Day>05</Day></PubMedPubDate><PubMedPubDate PubStatus="accepted"><Year>2020</Year><Month>08</Month><Day>10</Day></PubMedPubDate><PubMedPubDate PubStatus="entrez"><Year>2020</Year><Month>8</Month><Day>23</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate PubStatus="pubmed"><Year>2020</Year><Month>8</Month><Day>23</Day><Hour>6</Hour><Minute>0</Minute></PubMedPubDate><PubMedPubDate 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